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Center for Nanosystems Chemistry, Julius-Maximilians University Würzburg, Theodor Boveri-Weg 1, 97074 Würzburg, Germany and Institute for Physical and Theoretical Chemistry, Julius-Maximilians University Würzburg, Emil-Fischer Straße 42, 97074 Würzburg, Germany
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Charge-transfer states are revealed as key electronic gateways that mediate biexcitonic processes in molecular aggregates, offering a new perspective on singlet fission and exciton annihilation.