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Identifying 49 new high-energy methane transitions, including six previously unobserved states, reshapes our understanding of methane's spectral behavior at elevated temperatures.
Power broadening in Doppler-broadened double resonance spectroscopy is largely inhomogeneous, despite producing Lorentzian lineshapes, and saturation power is significantly lower than expected for homogeneous broadening.
Ethylene's hot-band transitions, previously unmeasured, are now characterized using optical frequency comb double-resonance spectroscopy, opening new avenues for understanding its vibrational energy levels.
