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Institute of Physics, University of Freiburg, Hermann-Herder-Stra脽e 3, 79104 Freiburg, Germany;
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Widely used approximations for modeling hot-exciton relaxation in semiconductor nanocrystals can fail, but mapping surface hopping (MASH) offers a more reliable alternative.
Negative electronic friction, often attributed to simple Joule heating, actually stems from significant non-Markovian effects that can destabilize standard Langevin descriptions of molecular dynamics.
